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Isotope effects in electron-impact dissociation of D2H+
2011,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross sections have been measured using the crossed electron–ion beams method for electron-impact dissociation of the D2H+ molecular ion yielding H+, D+, HD+ and D+2 fragments. The collision energy ranges from a few eV up to 2.5 keV. Around the maximum, cross sections are found to be of a similar amplitude: (3.25 ± 0.08) × 10−17 cm2 for H+, (3.56 ± 0.15) × 10−17 cm2 for HD+ and (3.33 ± 0.11) ...
Rotational dependence of the dipole moment of 13CH3F
2004,
- HENALLUX
,
- Article scientifique
Article scientifique
When a gas sample of 13CH3F is prepared with a population of spin isomers far from the equilibrium given by nuclear spin statistics, it relaxes towards this equilibrium with an exponential decay rate. This rate is increased by submitting the molecules to a static electric field, emphasizing the role of the magnetic intramolecular interactions and of the collisions in the “quantum relaxation” process ...
Absolute cross sections and kinetic energy release for doubly and triply charged fragments produced by electron impact on CO+
2006,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross sections for electron impact ionization of CO+ leading to the formation of doubly and triply charged products (CO2+, C2+ and O2+, C3+ and O3+) are reported in the energy range from their respective thresholds to 2500 eV. Around the maximum, cross section values are found to be (13.36 ± 0.56) × 10−18 cm2, (5.58 ± 0.55) × 10−18 cm2 and (1.37 ± 0.14) × 10−18 cm2 for CO2+, C2+ and O2+, ...
Electron impact multiple ionization of C+ and N+ and O+ ions
2014,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross sections for electron impact single and multiple ionization of C+, N+ and O+ ions leading to the formation of Cq+ (q=2-4), Nq+ (q=2-5) and Oq+ (q=2-5) are reported in the energy range extending from the respective thresholds up to 2.5 keV. The general feature of the measured cross sections is investigated.
A crossed-beam experiment for electron impact ionization and dissociation of molecular ions: its application to CO+
2006,
- HENALLUX
,
- Article scientifique
Article scientifique
A crossed electron–ion beam experimental set-up has been upgraded for the study of electron impact ionization and dissociation of molecular ions by means of ionic product detection. Both the experimental set-up and the data analysis procedures are described in detail for the estimation of (i) absolute cross sections, (ii) kinetic energy release distributions (KERD) and (iii) anisotropies of angular ...
Absolute cross sections and kinetic energy release distributions for electron-impact ionization and dissociation of CD+ 4
2008,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross sections for electron-impact dissociative excitation and ionization of CD+ 4 leading to formation of ionic products (CD2+ 4, CD+ 3, CD+ 2, CD+, C+, D+ 3, D+ 2, and D+) have been measured. The animated crossed-beams method is applied in the energy range from the reaction threshold up to 2.5 keV. Around 100 eV, the maximum cross sections are found to be (3.8±0.2) ×10-19 cm2, (10.8±1.5)× ...
Absolute cross-sections and kinetic-energy-release distributions for electron-impact ionization and dissociation of CD +3
2009,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross-sections have been measured for electron-impact dissociative excitation and ionization of CD+3/(CH+3) leading to formation of singly-charged fragments (CD +2, CH+, C+, H +2 and D+). The animated crossed-beams method is applied in the energy range from the reaction threshold up to 2.5 keV. The maximum cross-sections are found to be (14.0±1.0)×10-17 cm2, (6.5± 0.7)×10-17 cm2, (3.3± ...
Absolute cross-sections and kinetic-energy-release distributions for electron-impact ionization and dissociation of CD+ 2
2009,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross-sections have been measured for electron-impact dissociative excitation and ionization of CD +2 leading to formation of CD 2+2, CD+, C+, D +2 and D+. The animated crossed-beams method is applied in the energy range from the reaction threshold up to 2.5 keV. The maximum total cross-sections are found to be (1.2±0.1)×10-17 cm2, (6.1±0.7)×10-17 cm2, (6.4±0.7)×10-17 cm2, (26.3±3.8)×10-19 ...
Absolute cross sections and kinetic energy release distributions for electron impact ionization and dissociation of CD+
2007,
- HENALLUX
,
- Article scientifique
Article scientifique
Absolute cross sections for electron impact dissociative excitation and ionization of CD+ leading to the formation of ionic products (D+, C+, C2+ and C3+) are reported in the energy range from their respective thresholds to 2.5 keV. Around the maximum, cross sections are found to be (10.5 ± 1.0) × 10−17 cm2, (20.6 ± 3.5) × 10−17 cm2, (1.20 ± 0.11) × 10−17 cm2 and (8.2 ± 1.5) × 10−20 cm2 for D+, C+, ...
Nuclear spin conversion in the gaseous phase in the presence of a static electric field: Intramolecular magnetic interactions and the role of collisions
2004,
- HENALLUX
,
- Article scientifique
Article scientifique
When a gaseous sample of 13CH3F is prepared with a spin-isomer population ratio (ortho and para forms) far from the equilibrium given by nuclear spin statistics, it relaxes towards this equilibrium with an exponential decay rate. This phenomenon, called nuclear spin conversion, is mainly governed by intramolecular spin-spin and spin-rotation interactions which couple two pairs of quasidegenerate ...